New THz radiation devices made of high-Tc superconductors are fabricated and their characteristics are studied in detail. Ultrashort electromagnetic pulses with 0.5 ps width have been radiated into free space from current biased devices made of superconducting YBa2Cu3O7 (YBCO) films by exciting with femtosecond laser pulses. The Fourier spectrum of them extends up to 3 THz. The radiation mechanism is ascribed to the ultrafast supercurrent modulation by the optical pulses. The THz waveform is analyzed using rate equations describing the relaxation of photoexcited quasiparticles. By the improvement of the device structure and the collecting optics, the radiation power can be increased up to 0.5 µW. A new type THz radiation from YBCO films under an external magnetic field without a transport current is also reported.

The electric field intensity of the THz radiation from YBCO thin films excited by ultrashort laser pulses has been enhanced by a factor of 3 using a-axis oriented films instead of c-axis oriented ones used previously under the same excitation conditions. This corresponds to the enhancement of a factor of 10 for the radiation power. From the transmittance measurements of the millimeter wave for a-and c-axis oriented films, the origin of the enhancement is attributed to the increased fraction of the THz electromagnetic wave power transmitted from the YBCO film to free space. This result indicates that the utilization of the anisotropic properties of high-Tc superconductors is effective to enhance the radiation power.